No, all entries must have an absolute value less than 1.
If a unary matrix U has in entries uij then the ith diagonal elements of the product U U* is ui1*ui1*+ ui2*ui* + ... + uiN*uiN* = |ui1|2 +|ui2|2 + ... |uiN|2 = 1. So |uij|2 should be less or equal to 1 for each i and j.
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