The following changes would most improve his results: moving the magnet faster and using more loops of wire in the coil.
1. According to the Faraday's law, EMF in the loop is given by the rate of change of the magnetic flux:
"\\mathcal{E} = -\\dfrac{\\mathrm{d}\\Phi_B}{\\mathrm{d}t}" . Moving the magnet faster increases the speed of the magnetic flux changes and, thus, increases the current in the loop.
2. Again, according to the same Faraday's law:
"\\mathcal{E} = -N\\dfrac{\\mathrm{d}\\Phi_B}{\\mathrm{d}t}" , where "N" is number of coil turns. Using more loops of wire in the coil will also increse the EMF and, thus, the current in the wire.
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